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张岩

发布日期 :2022-04-14    阅读次数 :5151

基本信息


姓名:张 岩        职称:副教授

电子邮箱:zhangyan001@zjnu.edu.cn

职责:①浙师大化学学术型硕士研究生(化学)导师

    ②浙师大教师教育学院[教育硕士研究生(领域:学科教学)]导师

通讯地址:浙江金华迎宾大道688号浙江师范大学生化学院7401-D


教育经历

2012-092016-03,浙江大学,药学院,医学博士,导师:崔孙良教授

2008-092011-03,浙江大学,化学系,理学硕士,导师:商志才教授

2004-092008-07,曲阜师范大学,化学科学学院,理学学士


科研与学术工作经历

2019-092020-09,德国哥廷根大学,化学系,访问学者 (国家公派)

合作导师:Lutz Ackermann 教授

2018-12至今,浙江师范大学,化学与尊龙凯时平台入口,副教授

2016-042018-12,浙江师范大学,化学与尊龙凯时平台入口,讲师


研究方向

  1. 过渡金属催化的CH活化反应用于构建杂环化合物及生物活性分子

  2. 电氧化/还原下的自由基反应


主持项目

  1. Rh(III)催化非典型[4+2]环化构建中环内酰胺及多芳基乙烯分子骨架

国家自然科学基金青年项目(项目编号:21702188,已结题)

  1. 官能团化导向基辅助的Rh(III)催化用于构建环状化合物

浙江省自然科学基金青年项目(项目编号:LQ17B020001,已结题)

  1. 电氧化接力催化反应实现七元环化合物的简洁构建

浙江省自然科学基金一般项目(项目编号:LY22B020001,在研)


发表科研论文

  29. Yan Zhang,*Chunhang Zhao, Chanchan Ma, Zhenzhi Cai, Lutz Ackermann.*Photocatalytic C–C Cleavage of Methylenecyclobutanes for γ,δ-Unsaturated Aldehydes by Strain Release.Angew. Chem. Int. Ed. 2023, 62,DOI: 10.1002/anie.202300166.

    28. Yan Zhang,* Zhenzhi Cai, Chunhang Zhao, Hanliang Zheng, Lutz Ackermann.* Electrosynthesis of Bridged or Fused Sulfonamides through Complex Radical Cascade Reactions: Divergence in Medium-Sized Ring Formation. Chem. Sci. 2023, DOI: 10.10391D2SC07045F.

        27.Yan Zhang,Zhenzhi Cai, Svenja Warratz, Chanchan Ma, Lutz Ackermann. * Recent Advances in Electrooxidative Radical Transformations of Alkynes Sci. China Chem. 202366(3), 703-724. (IF2022 = 10.1)

26.Yan Zhang,* Chanchan Ma, Zhenzhi Cai, Julia Struwe, Shengjie Chen, Jinming Xu, Shiyin Li, Wangyu Zeng, Lutz Ackermann, "Electrooxidative tricyclic 6-7-6 fused-system domino assembly to allocolchicines by a removable radical strategy" Green Chem2022 24(9), 3697–3703. (IF2022 = 11.0)

25.Yan Zhang,* Zhenzhi Cai, Julia Struwe, Chanchan Ma, Wangyu Zeng, Xinyi Liao, Min Xu, Lutz Ackermann.*Dibenzocycloheptanones construction through a removable P-centered radical: Synthesis of allocolchicine analogues. Chem. Sci. 2021, 12, 15727–15732.PDF(IF2021 = 9.8)

24.Yan Zhang,*Chanchan Ma, Julia Struwe, Jian Feng, Gangguo Zhu, Lutz Ackermann.*Electrooxidative Dearomatization of Biaryls: Synthesis of Tri- and Difluoromethylated Spiro[5.5]trienones. Chem. Sci. 2021, 12, 10092–10096.PDF (IF = 9.8)

23.Yan Zhang,* ZhipengLin, Lutz Ackermann.* Electrochemical C–H Amidation of Heteroarenes with N-Alkyl Sulfonamides in Aqueous Medium.Chem. Eur. J. 2021, 27, 242–246. PDF

22.Yan Zhang, Julia Struwe, Lutz Ackermann.*Rhodium-Catalyzed Electrooxidative C–H Olefination of Benzamides. Angew. Chem. Int. Ed. 2020, 59, 15076–15080. (IF2021 = 15.3) PDF

21.Yan Zhang,* Chenchao Huang, Xinru Lin, Qi Hu, Boyue Hu, Gangguo Zhu. Modular Synthesis of Alkylarylazo Compounds via Iron(III)-Catalyzed Olefin Hydroamination. Org. Lett. 2019, 21, 2261–2264. (IF2019 = 6.6) PDF

20.Yan Zhang,* Haiqian Zhu, Yuting Huang, Qi Hu, Yu He, Yihang Wen and Gangguo Zhu. Multicomponebt Synthesis of Isoindolinones by RhIII Relay Catalysis: Synthesis of Pagoclone and Pazinaclone from Benzaldehyde.Org. Lett. 2019, 21, 1273–1277. (IF2019= 6.6) PDF

19.Yan Zhang,* Junhua Zhang, Boyue Hu, Mingming Ji, Shangyi Ye, Gangguo Zhu.* Synthesis of Difluoromethylated and PhosphoratedSpiro[5.5]trie-nones via Dearomative Spirocyclization of Biaryl Ynone. Org. Lett. 2018, 20, 2988–2992. (IF = 6.6) PDF

18.Yan Zhang,* Yu He, Lisha Li, Mingming Ji, Xiaozong, Li and Gangguo Zhu. Synthesis of Polyaryl Substituted Olefins via Rh(III)-Catalyzed One-Pot Reaction Using N-phenoxyacetamides, Ketones, and Hydrazines. J. Org. Chem. 2018, 83, 2898–2903. (IF2017 = 4.8) PDF

17.Yan Zhang,* Tianbo Shang, Lisha Li, Yu He, Tingting Wen, Yanan Tu, Shanshan Wang, Dan Lin. Rh(III)-catalyzed C–H activation-desymmetrization  of diazabicycles using enol as directing group: A straightforward approach to difunctionalized cyclopentenes. Tetrahedron Lett. 2018, 59, 1394. PDF

16.Yan Zhang,* Shangyi Ye, Mingming Ji, Lisha, Li, Dongmei Guo and Gangguo Zhu.Copper-Catalyzed Radical Cascade Difluoromethylation/ Cyclization of 2-(3-Arylpropioloyl)benzaldehydes: A Route to Difluoromethylated Naphthoquinones. J. Org. Chem. 2017,82,6811–6818.(IF2017 = 4.8) PDF

15.Yan Zhang,* Dongmei Guo, Shangyi Ye, Zhicheng Liu, Gangguo Zhu.* Synthesis of Trifluoromethylated Naphthoquinones via Copper-Catalyzed Cascade Trifluoromethylation/Cyclization of 2-(3-Arylpropioloyl) benzaldehydes. Org. Lett. 2017, 19, 1302–1305. (IF = 6.6) PDF

14.Hui Zhu, Weiwei Jin,Jiayao He,Yan Zhang,* Gangguo Zhu.*Synthesis of (E)-α,β-Unsaturated Carbonyls via Silver-Catalyzed Tandem Epoxide Rearrangement/Intermolecular Carbonyl-Heteroalkyne Metathesis, Advanced Synthesis & Catalysis. 2016, 358, 3730–3735. (IF = 5.45) PDF

13.Yan Zhang, Dahai Wang, Sunliang Cui.* Facile Synthesis of Isoindolinones via Rh(III)-Catalyzed One-Pot Reaction of Benzamides, Ketones, and Hydrazines. Org. Lett. 2015, 17, 2494–2497. (IF = 6.6) PDF

12.Yan Zhang, Mingyun Shen, Sunliang Cui,* Tingjun Hou. Synthesis and antiproliferative evaluation of 2-hydroxylated (E)-stilbenes. Bioorg. Med. Chem. Lett. 201424, 5470–5472. (IF = 2.45) PDF

11.Yan Zhang, Jing Zheng, Sunliang Cui.*Rh (III)-catalyzed C–H activation/ cyclization of indoles and pyrroles: divergent synthesis of heterocycles. J. Org. Chem. 2014, 79, 6490–6500. (IF = 4.75) PDF

10.Yan Zhang, Qifan Wu, Sunliang Cui.* Rh(III)-catalyzed C–H activation–desymmetrization of diazabicycles with arenes: facile synthesis of functionalized cyclopentenes. Chem. Sci. 2014, 5, 297–302. (IF = 9.6) PDF

9.Sunliang Cui,*Yan Zhang, Dahai Wang, Qifan Wu. Rh(III)-catalyzed C–H activation/[4 + 3] cycloaddition of benzamides and vinylcarbenoids: facile synthesis of azepinones. Chem. Sci. 2013, 4, 3912–3916. (IF2021 = 9.8) PDF

8.Sunliang Cui,*Yan Zhang, Qifan Wu. Rh(III)-catalyzed C–H activation /cycloaddition of benzamides and methylenecyclopropanes: divergence in ring formation. Chem. Sci. 2013, 4, 3421–3426. (IF2021 = 9.8) PDF

7.Yan Zhang, Xiang Chen, Jun Liang, Zhi-Cai Shang.* Room-Temperature Synthesis of Diindolylmethanes Using Silica-Supported Sulfuric Acid as a Reusable Catalyst Under Solvent-Free Conditions. Synth Commun. 2011, 41, 2446~2454. (IF2021 = 2.0) PDF

6.Yan Zhang, Hong Jin, Xinweng You, Zhi-Cai Shang.* A Novel, Green and Mild Access to Azole Heteroarenes:Synthesis of Pyrazoles in BrФnsted Acidic Ionic Liquid at Room Temperature. Chin. J. Org. Chem. 2011, 31, 387–391. PDF

5.Yan Zhang, Mei-Yuan Cheng, Zhi-Cai Shang.* Condensation Reactions between Aldehydes and 5,5-Dimethyl-1,3-cyclohexanedione in Water without Catalyst. Chin. J. Org. Chem. 2011, 31, 814–818. (IF = 1.3) PDF

4.Yan Zhang, Cui-Zhi Sun, Jun Liang, Zhi-Cai Shang.*Catalysis by L‐Lysine: A Green Method for the Condensation of Aromatic Aldehydes with Acidic Methylene Compounds in Water at Room Temperature. Chin. J. Chem. 2011, 28, 2255–2259. (IF2021 = 6.0) PDF

3.Yan Zhang, Zhi-Cai Shang.*A Green and Novel Method of Synthesizing 2,2′-Arylmethylene Bis(3-hydroxy-5,5-dimethylcyclohex-2-enone) Catalyzed by L-Histidine in Ionic Liquid. Chin. J. Chem. 2010, 28, 1184. (IF2021 = 6.0) PDF

2.Yan Zhang, Man-Gang Wang, Jun Liang, Zhi-Cai Shang.* An Environment-Friendly and Efficient Method for Aldol Condensation Catalyzed by L-Lysine in Pure Water. Lett. Org. Chem. 2010, 7, 27–31. PDF

1.Yan Zhang, Jun Liang, Zhi-Cai Shang.*Fast and Eco-friendly Synthesis of Dipyrromethanes by H2SO4·SiO2 Catalysis under Solvent-Free Conditions. Chin. J. Chem.2010, 28, 259–262. (IF2021 = 6.0) PDF


申请发明专利

9Yan Zhang  Method for preparing compound with spiro[5.5] molecular skeleton by electrooxidation  Patent No.: US 11,414,768 B1

8张岩,曾王玉,陈聖杰,徐斤铭,徐敏,涂凤,廖心怡,马婵婵,蔡圳枝,王依萌:一种电氧化条件下自由基串联环化合成二苯并环庚酮衍生物的方法,中国,专利号:ZL 202111418200.5

7.张岩,马婵婵,李诗音,陈圣杰,廖心怡,张莹,吴珍珍,黄朝漫:一种电氧化氟化制备螺[5.5]分子骨架类化合物的方法,中国,专利号:ZL 202110309275.3

6.张岩,黄朝漫,吴珍珍,施旋,吴潇逸,高喜玲:一种通过自由基环化反应构建二苯并环庚酮骨架的方法,中国,专利号:ZL20201102265.4

5.张岩,高喜玲,林心如:一种芳香酰胺类化合物的邻位烯基化方法,中国, 授权专利号:ZL 202010083526.6

4.张岩,林心如,黄玉婷,胡琦,胡博跃,何宇,朱钢国:一种抗焦虑药物帕戈隆或帕秦克隆的制备方法,中国,授权专利号:ZL 201811437849.X

3.张岩,朱钢国,黄玉婷,胡琦,陈李琼,胡雅卿:一种芳基烷基取代的偶氮类化合物的合成方法,中国,授权专利号:ZL 2018 1 1182978.9

2.张岩,朱钢国,朱海倩,黄晨超,戚佳一,陈泽辉:一种Rh(III)催化具有氮杂环骨架的化合物的制备方法,中国,授权专利号:ZL 201811178105.0

1.崔孙良张岩,侯廷军:反式邻羟基二苯乙烯衍生物及其制备方法和应用,中国, 授权专利号:ZL 201410432114.3


曾获荣誉

13.浙江省第十三届大学生化学竞赛获二等奖(2022,指导教师)

12.第三届全国大学生化学实验创新设计大赛“微瑞杯”华东赛区竞赛二等奖(2022年,指导老师)

11.浙江省第十二届大学生化学竞赛获一等奖(2021,指导教师,两项)

10.浙江师范大学第十三届青年教师教学竞赛获优胜奖(2021年)

9.浙师大生化学院青年教师教学技能比赛二等奖(2021年)

8.浙江省第十六届“挑战杯”大学生课外科技竞赛三等奖(2019,指导老师)

7.浙师大生化学院青年教师教学技能比赛三等奖(2019年)

6.浙江师范大学优秀班主任(2018

5.浙江省第九届大学生化学竞赛一等奖(2017,指导教师)

4.浙江省优秀毕业生(2016年)

3.浙江大学“三好研究生” (2013-2015,连续三次)

2.博士研究生国家奖学金(2014年)

1.山东省优秀毕业生(2008年)


教学改革项目、论文及指导学生

1.浙江师范大学教学改革项目(课堂教学改革专题)(2021年,负责人):关于《有机合成/实验》课堂教学中存在的若干问题的思考

2.浙师大生化学院课堂教学改革项目(2020年,负责人):实践中印证理论,将企业实际生产项目带入课堂——以《有机合成/实验》为例

3.胡博跃,高喜玲,林心如,张岩,胡琦,黄玉婷:一种电氧化胺化制备2-氨基吲哚类化合物的方法,中国, 专利号:202010193576.X。(本科生第一发明人)

4.Shiyin Li #, Xinru Lin#, Xiling Gao#, Wangyu Zeng, Xiaoyi Wu, Xuan Shi, Shengjie Chen, and Yan Zhang.*Uncatalyzed Synthesis of Unsymmetrical Indole- substituted Methane Derivatives via One-pot Multicomponent Reactions under Solvent-Free Conditions. Lett. Org. Chem. 2022, 19, 190-197.(本科生第一作者)

5.林心如,乔元皇,李诗音,张岩*. 含有手性碳原子的有机分子R/S构型的快速判断方法. 教育现代化,2021,8 (77), 74-78。(本科生第一作者论文)

6.张岩,* 吴潇逸,高喜玲,张莹,涂凤. 基于深度学习理论的有机合成课程教学改革. 化学教育(中英文,北大核心),202243(10),35-40。

7.张岩,* 吴潇逸,吴阳,高喜玲. 基于深度学习理论的有机重排反应课堂教学.大学化学2022,DOI:10.3866/PKU.DXHX202209060

8.国家大学生创新创业训练项目(国创),3项(2017, 2018 , 2020年,都已结题)

 浙江省大学生科技创新项目(新苗),2项(2021, 2022年)

9.浙江省优秀毕业研究生 马婵婵 2023


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